Gaming - no.
Workstation - depends on the work. I can imagine that compiles of large systems speed up by a couple of percent. Putting your Chrome profile on one could be beneficial. I have my gaming machine Windows boot on Optane but never measured whether it actually does anything faster.
mdadm is very good software but since it separates filesystem and raid it has the "raid hole". Not their fault but a disadvantage nontheless.
Never ran btrfs and probably never will.
RAID6 is absolutely worth it over RAiD5. The problem is that after a drive failure you rsync a new drive. And the resync puts a lot of stress on the remaining old drives. At a time where one more drive failure takes your array offline.
As for OS, I would use ZFS on FreeBSD, possibly inside Proxmox.
It's actually pretty hard/annoying to track down any many-disks chassis lately. I'm still feeding off Cooler Master Stacker 810 cases that I bought ca. 2005.
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